| Year | Actor or Actress | Film |
| 2008 | Arjun Rampal | Om Shanti Om |
| 2007 | Saif Ali Khan | Omkara |
| 2006 | Nana Patekar | Apaharan |
| 2005 | John Abraham | Dhoom |
| 2004 | Rahul Dev | Footpath |
| 2003 | Ajay Devgan | Deewangee |
| 2002 | Aftab Shivdasani | Kasoor |
| 2001 | Sushant Singh | Jungle |
| 2000 | Ashutosh Rana | Sangharsh |
| 1999 | Ashutosh Rana | Dushman |
| 1998 | Kajol | Gupt |
Zee Cine Awards For Best Villain
The Zee Cine Awards for Best Villain is chosen by a jury organized by Zee Entertainment Enterprises and is awarded to an actor or actress who portrayed the role of an antagonist. The first actress to win this award was Kajol for her role in ‘Gupt’.
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